In the past the Sysinternals Suite used to have only a few 64-bit versions of their tools, but recently they added many more.
The documentation doesn’t reflect this yet, but the online versions do:
These are 64-bit:
Wednesday, June 29, 2016 9:42 PM 403120 accesschk64.exe
Wednesday, June 29, 2016 9:42 PM 841904 Autoruns64.exe
Wednesday, June 29, 2016 9:42 PM 742064 autorunsc64.exe
Wednesday, June 29, 2016 9:42 PM 154792 Clockres64.exe
Wednesday, June 29, 2016 9:42 PM 268960 Contig64.exe
Wednesday, June 29, 2016 9:42 PM 158376 diskext64.exe
Wednesday, June 29, 2016 9:42 PM 190104 du64.exe
Wednesday, June 29, 2016 9:42 PM 169136 FindLinks64.exe
Wednesday, June 29, 2016 9:42 PM 226464 handle64.exe
Wednesday, June 29, 2016 9:42 PM 164520 hex2dec64.exe
Wednesday, June 29, 2016 9:42 PM 236200 junction64.exe
Wednesday, June 29, 2016 9:43 PM 220336 Listdlls64.exe
Wednesday, June 29, 2016 9:43 PM 156840 LoadOrd64.exe
Wednesday, June 29, 2016 9:43 PM 188584 LoadOrdC64.exe
Wednesday, June 29, 2016 9:43 PM 249536 logonsessions64.exe
Wednesday, June 29, 2016 9:43 PM 154792 movefile64.exe
Wednesday, June 29, 2016 9:43 PM 265904 notmyfault64.exe
Wednesday, June 29, 2016 9:43 PM 271032 notmyfaultc64.exe
Wednesday, June 29, 2016 9:43 PM 158896 ntfsinfo64.exe
Wednesday, June 29, 2016 9:43 PM 156336 pendmoves64.exe
Wednesday, June 29, 2016 9:43 PM 234160 pipelist64.exe
Thursday, April 28, 2016 12:25 AM 310440 procdump64.exe
Wednesday, June 29, 2016 9:43 PM 374944 PsExec64.exe
Wednesday, June 29, 2016 9:43 PM 168608 psfile64.exe
Wednesday, June 29, 2016 9:43 PM 326824 PsGetsid64.exe
Wednesday, June 29, 2016 9:43 PM 351912 PsInfo64.exe
Wednesday, June 29, 2016 9:43 PM 318624 pskill64.exe
Wednesday, June 29, 2016 9:43 PM 202400 pslist64.exe
Wednesday, June 29, 2016 9:43 PM 170160 PsLoggedon64.exe
Wednesday, June 29, 2016 9:43 PM 168616 pspasswd64.exe
Wednesday, June 29, 2016 9:43 PM 293032 psping64.exe
Wednesday, June 29, 2016 9:43 PM 210608 PsService64.exe
Wednesday, June 29, 2016 9:43 PM 321704 pssuspend64.exe
Wednesday, June 29, 2016 9:43 PM 164024 RegDelNull64.exe
Wednesday, June 29, 2016 9:43 PM 160400 ru64.exe
Wednesday, June 29, 2016 9:43 PM 165544 sdelete64.exe
Wednesday, June 29, 2016 9:43 PM 856752 sigcheck64.exe
Wednesday, June 29, 2016 9:43 PM 153768 streams64.exe
Wednesday, June 29, 2016 9:43 PM 162472 strings64.exe
Wednesday, June 29, 2016 9:43 PM 158360 sync64.exe
Thursday, April 28, 2016 12:25 AM 862888 Sysmon64.exe
Tuesday, February 2, 2016 10:04 PM 221360 Testlimit64.exe
Wednesday, June 29, 2016 9:43 PM 169648 Volumeid64.exe
Wednesday, June 29, 2016 9:43 PM 169632 whois64.exe
These do not have 64-bit equivalents yet or (like procexp.exe) have 64-bit versions embedded (some will likely never get them):
Wednesday, November 1, 2006 1:06 PM 174968 AccessEnum.exe
Wednesday, November 14, 2012 10:22 AM 479832 ADExplorer.exe
Tuesday, October 27, 2015 12:13 AM 2425496 ADInsight.exe
Wednesday, November 1, 2006 1:05 PM 150328 adrestore.exe
Tuesday, February 22, 2011 2:18 PM 148856 Autologon.exe
Tuesday, October 27, 2015 11:28 PM 2049168 Bginfo.exe
Wednesday, November 1, 2006 1:06 PM 154424 Cacheset.exe
Monday, August 18, 2014 7:29 PM 892088 Coreinfo.exe
Wednesday, November 1, 2006 1:05 PM 150328 ctrl2cap.exe
Monday, December 3, 2012 10:10 AM 468056 Dbgview.exe
Wednesday, November 1, 2006 9:06 PM 158520 DEFRAG.EXE
Wednesday, October 17, 2012 5:28 PM 116824 Desktops.exe
Wednesday, November 1, 2006 1:06 PM 224056 Diskmon.exe
Wednesday, March 24, 2010 1:00 PM 580984 DiskView.exe
Wednesday, May 20, 2015 2:24 AM 146232 efsdump.exe
Wednesday, November 1, 2006 1:06 PM 154424 ldmdump.exe
Tuesday, December 17, 2013 4:01 PM 559808 livekd.exe
Wednesday, November 1, 2006 1:06 PM 215928 pagedfrg.exe
Friday, January 13, 2012 4:35 PM 451392 portmon.exe
Thursday, February 4, 2016 10:19 PM 2694816 procexp.exe
Friday, June 12, 2015 12:34 AM 2046608 Procmon.exe
Tuesday, April 27, 2010 10:04 AM 178040 psloglist.exe
Monday, December 4, 2006 4:53 PM 207664 psshutdown.exe
Tuesday, February 2, 2016 10:04 PM 625816 RAMMap.exe
Wednesday, November 1, 2006 9:05 PM 146232 Reghide.exe
Tuesday, February 2, 2016 10:04 PM 117920 regjump.exe
Wednesday, November 1, 2006 1:07 PM 334720 RootkitRevealer.exe
Wednesday, November 1, 2006 1:07 PM 260976 ShareEnum.exe
Wednesday, February 27, 2008 5:51 PM 103464 ShellRunas.exe
Wednesday, July 28, 2010 2:47 PM 199544 tcpvcon.exe
Monday, July 25, 2011 11:40 AM 300832 Tcpview.exe
Monday, July 20, 2015 11:45 PM 1194128 vmmap.exe
Tuesday, June 18, 2013 2:12 PM 596160 ZoomIt.exe
–jeroen